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Abstract
Solution-processed quantum-dot light-emitting diodes (QLEDs) suffer from shelf-stability issues due to the ZnO-induced positive aging effect. This paper presents a bilayer electron-transporting layer (ETL) design using SnO₂ nanoparticles (NPs) as a buffer layer between the quantum dots (QDs) and ZnO NPs. This design suppresses QD-ETL exciton quenching, tunes charge balance, and maintains high electron conductivity. The resulting bottom-emitting QLEDs achieve a maximum luminance exceeding 100,000 cd m⁻² and a T₉₅ operational lifetime of 6200 h at 1000 cd m⁻², while completely inhibiting positive aging.
Publisher
npj Flexible Electronics
Published On
Jan 31, 2022
Authors
Zi Ye, Mengyu Chen, Xingtong Chen, Wenchen Ma, Xiaojuan Sun, Longjia Wu, Xiongfeng Lin, Yu Chen, Song Chen
Tags
QLEDs
electron-transporting layer
SnO₂ nanoparticles
ZnO
charge balance
luminance
operational lifetime
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