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Abstract
This paper proposes methyl formate (MF) as a novel hydrogen storage material. Utilizing appropriate catalysts, hydrogen production from MF is significantly faster than with other established chemical hydrogen carriers under mild conditions. The optimized system shows high activity (TOFmax > 44,000 h−1 and TON > 100,000) and selectivity (undetectable CO). Solvent-free dehydrogenation demonstrates its application potential.
Publisher
Nature Catalysis
Published On
Jun 22, 2023
Authors
Rui Sang, Zhihong Wei, Yuya Hu, Elisabetta Alberico, Duo Wei, Xinxin Tian, Pavel Ryabchuk, Anke Spannenberg, Rauf Razzaq, Ralf Jackstell, Jonas Massa, Peter Sponholz, Haijun Jiao, Henrik Junge, Matthias Beller
Tags
hydrogen storage
methyl formate
dehydrogenation
catalysts
clean energy

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