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An efficient approach to angular tricyclic molecular architecture via Nazarov-like cyclization and double ring-expansion cascade

Chemistry

An efficient approach to angular tricyclic molecular architecture via Nazarov-like cyclization and double ring-expansion cascade

Y. Wang, K. Fang, et al.

Explore a groundbreaking method for creating angular tri-carbocyclic architectures featuring quaternary carbon centers, achieved through a unique Nazarov cyclization and ring expansions. This innovative approach, characterized by high selectivity and mild conditions, enables a racemic total synthesis of (±)-waihoensene in just 18 steps, all thanks to the collaborative research by Yun-Peng Wang, Kun Fang, Yong-Qiang Tu, Jun-Jie Yin, Qi Zhao, and Tian Ke.

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