Sustainable production of hydrogen with high purity from | ResearchBunny

Index

Abstract

This paper demonstrates that dual-active sites of Pt single-atoms and frustrated Lewis pairs (FLPs) on porous nanorods of CeO₂ enable efficient, additive-free H₂ generation with low CO (0.027%) through aqueous-phase reforming of methanol (APRM) at 120 °C. Pt single-atoms and Lewis acidic sites cooperatively activate methanol, while spontaneous water dissociation on FLPs improves CO reforming, boosting H₂ production and suppressing CO generation. This offers a promising path for flexible hydrogen utilization.

Publisher

Nature Communications

Published On

Sep 21, 2022

Authors

Sai Zhang, Yuxuan Liu, Mingkai Zhang, Yuanyuan Ma, Jun Hu, Yongquan Qu

Related Publications

Explore these studies to deepen your understanding of the subject.

Engineering and Technology

Production of hydrogen from offshore wind in China and cost-competitive supply to Japan

S. Song, H. Lin, et al.

Medicine and Health

Low Omega-3 intake is associated with high rates of depression and preterm birth on the country level

T. H. Ciesielski and S. M. Williams

Economics

The impact of economic freedom on economic growth in countries with high and low regulatory quality—lessons for Viet Nam

N. T. Hung, T. T. K. Oanh, et al.

Education

Writing impact case studies: a comparative study of high-scoring and low-scoring case studies from REF2014

B. Reichard, M. S. Reed, et al.

Listen, Learn & Level Up

Over 10,000 hours of research content in 25+ fields, available in 12+ languages.

No more digging through PDFs—just hit play and absorb the world's latest research in your language, on your time.

listen to research audio papers with researchbunny