This paper reports the design and fabrication of a conductive adhesive-barrier (CAB) for halide perovskite-based photoelectrochemical cells, achieving record solar-to-hydrogen (STH) efficiencies. A co-planar architecture reached 13.4% STH efficiency, while a monolithic stacked silicon-perovskite tandem achieved 20.8% STH efficiency with 102 h of operation. This advance contributes to efficient, durable, and low-cost solar-driven water-splitting technology.
Publisher
Nature Communications
Published On
Jun 26, 2023
Authors
Austin M. K. Fehr, Ayush Agrawal, Faiz Mandani, Christian L. Conrad, Qi Jiang, So Yeon Park, Olivia Alley, Bor Li, Siraj Sidhik, Isaac Metcalf, Christopher Botello, James L. Young, Jacky Even, Jean Christophe Blancon, Todd G. Deutsch, Kai Zhu, Steve Albrecht, Francesca M. Toma, Michael Wong, Aditya D. Mohite
Tags
conductive adhesive-barrier
solar-to-hydrogen efficiency
photoelectrochemical cells
halide perovskites
water-splitting technology
sustainable energy
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