The Mott insulator Ca₂RuO₄ exhibits an insulator-to-metal transition induced by d.c. current. This study uses transport-ARPES to probe the electronic structure under current, revealing a clear reduction of the Mott gap and a modification in the Ru band dispersion. A free-energy analysis shows the current-induced phase is distinct from the high-temperature metallic phase, highlighting the interplay between lattice and orbital-dependent electronic responses in the current-driven transition.
Publisher
Nature Physics
Published On
Sep 24, 2024
Authors
C. T. Suen, I. Marković, M. Zonno, N. Heinsdorf, S. Zhdanovich, N. H. Jo, M. Schmid, P. Hansmann, P. Puphal, K. Fürsich, S. Smit, C. Au-Yeung, V. Zimmermann, B. Zwartsenberg, M. Krautloher, I. S. Elfimov, R. Koch, S. Gorovikov, C. Jozwiak, A. Bostwick, M. Franz, Eli Rotenberg, B. Keimer, A. Damascelli
Tags
Mott insulator
Ca₂RuO₄
insulator-to-metal transition
d.c. current
transport-ARPES
Mott gap
band dispersion
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