logo
ResearchBunny Logo
Abstract
This paper presents a novel photon-phonon-driven cascade reaction for converting methane to formaldehyde with high productivity (401.5 µmol h⁻¹) and selectivity (90.4%) at 150 °C. A ZnO catalyst decorated with single Ru atoms facilitates a two-step process: photocatalytic production of methyl hydroperoxide followed by its thermodecomposition into formaldehyde. Single Ru atoms enhance charge separation and oxygen reduction, leading to improved efficiency and minimizing energy consumption.
Publisher
Nature Sustainability
Published On
Sep 01, 2024
Authors
Youxun Xu, Chao Wang, Xiyi Li, Lunqiao Xiong, Tianyu Zhang, Liquan Zhang, Qinghua Zhang, Lin Gu, Yang Lan, Junwang Tang
Tags
photon-phonon-driven
cascade reaction
methane conversion
formaldehyde
ZnO catalyst
single Ru atoms
energy efficiency

Related Publications

Explore these studies to deepen your understanding of the subject.

An efficient approach to angular tricyclic molecular architecture via Nazarov-like cyclization and double ring-expansion cascade
Chemistry

An efficient approach to angular tricyclic molecular architecture via Nazarov-like cyclization and double ring-expansion cascade

Y. Wang, K. Fang, et al.

Water enables mild oxidation of methane to methanol on gold single-atom catalysts
Chemistry

Water enables mild oxidation of methane to methanol on gold single-atom catalysts

L. Luo, J. Luo, et al.

Economically viable co-production of methanol and sulfuric acid via direct methane oxidation
Chemistry

Economically viable co-production of methanol and sulfuric acid via direct methane oxidation

J. Im, S. Cheong, et al.

Chronic exposure to synthetic food colorant Allura Red AC promotes susceptibility to experimental colitis via intestinal serotonin in mice
Medicine and Health

Chronic exposure to synthetic food colorant Allura Red AC promotes susceptibility to experimental colitis via intestinal serotonin in mice

Y. H. Kwon, S. Banskota, et al.

Listen, Learn & Level Up
Over 10,000 hours of research content in 25+ fields, available in 12+ languages.
No more digging through PDFs—just hit play and absorb the world's latest research in your language, on your time.
listen to research audio papers with researchbunny