This paper demonstrates a dynamic dual pattern using a supramolecular network for bilayer wrinkling systems. Both wrinkle morphology and fluorescence color are simultaneously regulated by visible light-triggered isomerization or acids. The resulting hierarchical patterned surface reversibly changes between smooth and wrinkled states, with fluorescence shifting from blue to orange-red. This smart surface with dynamic hierarchical wrinkles and fluorescence has potential anticounterfeiting applications.
